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    Solubility of uranium and thorium from a healing earth in synthetic gut fluids: A case study for use in dose assessments.
        
        Sci. Total Environ. 408, 5794-5800 (2010)
    
    
    
				The aim of this case study was to estimate the bioaccessibility of uranium ((238)U) and thorium ((232)Th) from a healing earth by analysing the solubility of these radionuclides in synthetic gastric and intestinal fluids. An easy applicable in vitro test system was used to investigate the fractional mobilization of the soil contaminants being potentially available for absorption under human in vivo conditions. These findings provided the basis for a prospective dose assessment. The solubility experiments were performed using two different in vitro digestion methods. The concentrations of (238)U and (232)Th in the solutions extracted from the soil were measured by inductively coupled plasma mass spectrometry (ICP-MS). The dissolved fractions in the synthetic gastrointestinal fluid ranged in average from 10.3% to 13.8% for (238)U and from 0.3% to 1.6% for (232)Th, respectively, depending on the digestion method. Subsequently, the committed effective doses from intake of (238)U and (232)Th after ingestion of the healing earth during 1 year were evaluated for adult persons. Thereby ingestion dose coefficients calculated as a function of bioaccessibility were used. The dose assessments ranged between 4.3×10(-7)-1.9×10(-6) Sv y(-1) for (238)U and 5.6×10(-7)-3.3×10(-6) Sv y(-1) for (232)Th, respectively. On the basis of the assumptions and estimations made, the present work indicates a relatively low radiation risk due to (238)U and (232)Th after internal exposure of the healing earth.
			
			
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Times Cited
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Scopus
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					Cited By
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        Publikationstyp
        Artikel: Journalartikel
    
 
    
        Dokumenttyp
        Wissenschaftlicher Artikel
    
 
     
    
    
        Schlagwörter
        Uranium; Thorium; Bioaccessibility; Soil; Ingestion; Dose assessments
    
 
     
    
    
        Sprache
        englisch
    
 
    
        Veröffentlichungsjahr
        2010
    
 
     
    
        HGF-Berichtsjahr
        2010
    
 
    
    
        ISSN (print) / ISBN
        0048-9697
    
 
    
        e-ISSN
        1879-1026
    
 
     
     
     
	     
	 
	 
    
        Zeitschrift
        Science of the Total Environment, The
    
 
		
    
        Quellenangaben
        
	    Band: 408,  
	    Heft: 23,  
	    Seiten: 5794-5800 
	    
	    
	
    
 
  
         
        
            Verlag
            Elsevier
        
 
         
	
         
         
         
         
         
	
         
         
         
    
         
         
         
         
         
         
         
    
        Begutachtungsstatus
        Peer reviewed
    
 
    
        Institut(e)
        Research Unit Medical Radiation Physics and Diagnostics (AMSD)
Institute of Radiation Protection (ISS)
 
    Institute of Radiation Protection (ISS)
        POF Topic(s)
        30504 - Mechanisms of Genetic and Environmental Influences on Health and Disease
    
 
    
        Forschungsfeld(er)
        Radiation Sciences
    
 
    
        PSP-Element(e)
        G-503600-001
G-501100-002
 
     
     	
    G-501100-002
        PubMed ID
        20832099
    
    
    
        Scopus ID
        77958110834
    
    
        Erfassungsdatum
        2010-10-27