PuSH - Publication Server of Helmholtz Zentrum München: Surface catalyzed halogenation-dehalogenation reactions of aromatic bromine compounds adsorbed on fly ash.

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Zier, B. ; Lenoir, D. ; Lahaniatis, E.S. ; Kettrup, A.

Surface catalyzed halogenation-dehalogenation reactions of aromatic bromine compounds adsorbed on fly ash.

Chemosphere 22, 1121-1129 (1991)

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Open Access Gold as soon as Publ. Version/Full Text is submitted to ZB.

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Brominated aromatic compounds like brominated benzenes, diphenylethers and dibenzodioxins adsorbed on the surface of fly ash from a municipal waste incininerator give mixed brominated/chlorinated und completely chlorinated aromatic compounds. These consecutive halogenation-dehalogenation reactions proceed by a nucleophilic mechanism, which is favoured by a high concentration of chloride on the fly ash. Results of kinetic and stereoselective behavior of these reactions will be discussed. The relevance of these results for PCDD/PCDF formation from bromine precursors in municipal waste incinerators will be discussed.

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