PuSH - Publication Server of Helmholtz Zentrum München

Export: TXT Text RIS Endnote (RIS) BIB BibTeX
Martens, P.* ; Czech, H. ; Orasche, J. ; Abbaszade, G. ; Sklorz, M. ; Michalke, B. ; Tissari, J.* ; Bizjak, T.* ; Ihalainen, M.* ; Suhonen, H.* ; Yli-Pirilä, P.* ; Jokiniemi, J.* ; Sippula, O.* ; Zimmermann, R.

Brown coal and logwood combustion in a modern heating appliance: The impact of combustion quality and fuel on organic aerosol composition.

Environ. Sci. Technol. 57, 5532-5543 (2023)
Publ. Version/Full Text DOI PMC
Closed
Open Access Green as soon as Postprint is submitted to ZB.
Residential heating with solid fuels is one of the major drivers for poor air quality in Central and Eastern Europe, and coal is still one of the major fuels in countries, such as Poland, the Czech Republic, and Hungary. In this work, emissions from a single-room heater fueled with brown coal briquettes (BCBs) and spruce logs (SLs) were analyzed for signatures of inorganic as well as semivolatile aromatic and low-volatile organic constituents. High variations in organic carbon (OC) emissions of BCB emissions, ranging from 5 to 22 mg MJ-1, were associated to variations in carbon monoxide (CO) emissions, ranging from 900 to 1900 mg MJ-1. Residential BCB combustion turned out to be an equally important source of levoglucosan, an established biomass burning marker, as spruce logwood combustion, but showed distinct higher ratios to manosan and galactosan. Signatures of polycyclic aromatic hydrocarbons emitted by BCB combustion exhibited defunctionalization and desubstitution with increasing combustion quality. Lastly, the concept of island and archipelago structural motifs adapted from petroleomics is used to describe the fraction low-volatile organic compounds in particulate emissions, where a transition from archipelago to island motifs in relation with decreasing CO emissions was observed in BCB emissions, while emissions from SL combustion exhibited the island motif.
Impact Factor
Scopus SNIP
Web of Science
Times Cited
Scopus
Cited By
Altmetric
11.400
0.000
1
1
Tags
Annotations
Special Publikation
Hide on homepage

Edit extra information
Edit own tags
Private
Edit own annotation
Private
Hide on publication lists
on hompage
Mark as special
publikation
Publication type Article: Journal article
Document type Scientific Article
Keywords Biomass Burning ; Levoglucosan ; Lignite ; Photoionization ; Residential Wood Combustion; Polycyclic Aromatic-hydrocarbons; Flight Mass-spectrometry; Emission Factors; Wood Combustion; Air-pollution; Carbonaceous Particles; Particulate Matter; Household Stoves; Pyrolysis; Biomass
Language english
Publication Year 2023
HGF-reported in Year 2023
ISSN (print) / ISBN 0013-936X
e-ISSN 1520-5851
Journal Environmental Science & Technology
Quellenangaben Volume: 57, Issue: 14, Pages: 5532-5543 Article Number: , Supplement: ,
Publisher ACS
Publishing Place Washington, DC
Reviewing status Peer reviewed
Institute(s) Cooperation Group Comprehensive Molecular Analytics (CMA)
Research Unit BioGeoChemistry and Analytics (BGC)
POF-Topic(s) 30202 - Environmental Health
Research field(s) Environmental Sciences
PSP Element(s) G-504500-001
G-504800-002
Grants Academy of Finland (AKA)
Academy of Finland
Helmholtz Virtual Institute of Complex Molecular Systems in Environmental Health (HICE)
Helmholtz Association of German Research Centres (HGF) within the Helmholtz International Lab aeroHEALTH
DOI 10.1021/acs.est.2c08787
WOS ID 000970541700001
Scopus ID 85151381239
PubMed ID 36976662
Erfassungsdatum 2023-10-06
[➜Report correction]