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Eshetu, G.G.* ; Zhang, H.* ; Judez, X.* ; Adenusi, H.* ; Armand, M.* ; Passerini, S.* ; Figgemeier, E.*

Production of high-energy Li-ion batteries comprising silicon-containing anodes and insertion-type cathodes.

Nat. Commun. 12:5459 (2021)

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Rechargeable Li-based battery technologies utilising silicon, silicon-based, and Si-derivative anodes coupled with high-capacity/high-voltage insertion-type cathodes have reaped significant interest from both academic and industrial sectors. This stems from their practically achievable energy density, offering a new avenue towards the mass-market adoption of electric vehicles and renewable energy sources. Nevertheless, such high-energy systems are limited by their complex chemistry and intrinsic drawbacks. From this perspective, we present the progress, current status, prevailing challenges and mitigating strategies of Li-based battery systems comprising silicon-containing anodes and insertion-type cathodes. This is accompanied by an assessment of their potential to meet the targets for evolving volume- and weight-sensitive applications such as electro-mobility.

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